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Unveiling a Recycling-Sourced Mineral-Biocellulose Fibre Composite for Use in Combustion-Generated NOx Mitigation Forming Plant Nutrient: Meeting Sustainability Development Goals in the Circular Economy

Thumbnail
2020
applsci-10-03927-v2.pdf (17.57Mb)
Authors
Gane, Patrick
Dimić-Misić, Katarina
Barać, Nemanja
Imani, Monireh
Janaćković, Đorđe
Uskoković, Petar
Barcelo, Ernest
Article (Published version)
Metadata
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Abstract
Featured Application Surface flow filter for sorption of NOx in city/industrial pollution and conversion into a plant nutrient. Abstract NOx is unavoidably emitted during combustion in air at high temperature and/or pressure, which, if exceeding recommended levels, has a negative impact on the population. The authors found that when moist, limestone (CaCO3) readily sorbs NO2 to form calcium nitrate, which provides the basis for developing a surface flow filter. The substrate was made from "over-recycled" cellulose fibres such as newsprint, magazines, or packaging fibre, which are too weak to be used in further recycling. The substrate was specially-coated with fine-ground calcium carbonate and micro-nano-fibrillated cellulose, which was used as a binder and essential humectant to avoid formation of a stagnant air layer. Pre-oxidation countered the action of denitrification bacteria colonising the cellulose substrate. The by-product CO2 produced in situ during carbonate to nitrate conve...rsion was adsorbed by perlite, which is an inert high surface-area additive. After use, the nitrate-rich CaCO3-cellulose-based filter was proposed to be mulched into a run-off resistant soil fertiliser and micronutrient suitable, e.g., for renewable forestry within the circular economy. Belgrade, Serbia, which is a highly polluted city, was used as a laboratory test bed, and NO2 was successfully removed from an inlet of city air. A construct of street-side self-draughting or municipal/commercial transport vehicle-exterior motion-draught filter boxes is discussed.

Keywords:
NOx sorption / gaseous pollution mitigation / cellulose circular economy / micro-nano-fibrillated cellulose humectant / sustainable energy solutions / zero carbon transport / zero carbon combustion systems
Source:
Applied Sciences-Basel, 2020, 10, 11
Publisher:
  • MDPI, Basel
Funding / projects:
  • Omya International AG, Group Sustainability

DOI: 10.3390/app10113927

WoS: 000543385900264

Scopus: 2-s2.0-85087012875
[ Google Scholar ]
3
3
URI
http://TechnoRep.tmf.bg.ac.rs/handle/123456789/4529
Collections
  • Radovi istraživača (Inovacioni centar) / Researchers’ publications (Innovation Centre)
  • Radovi istraživača / Researchers’ publications (TMF)
Institution/Community
Tehnološko-metalurški fakultet
TY  - JOUR
AU  - Gane, Patrick
AU  - Dimić-Misić, Katarina
AU  - Barać, Nemanja
AU  - Imani, Monireh
AU  - Janaćković, Đorđe
AU  - Uskoković, Petar
AU  - Barcelo, Ernest
PY  - 2020
UR  - http://TechnoRep.tmf.bg.ac.rs/handle/123456789/4529
AB  - Featured Application Surface flow filter for sorption of NOx in city/industrial pollution and conversion into a plant nutrient. Abstract NOx is unavoidably emitted during combustion in air at high temperature and/or pressure, which, if exceeding recommended levels, has a negative impact on the population. The authors found that when moist, limestone (CaCO3) readily sorbs NO2 to form calcium nitrate, which provides the basis for developing a surface flow filter. The substrate was made from "over-recycled" cellulose fibres such as newsprint, magazines, or packaging fibre, which are too weak to be used in further recycling. The substrate was specially-coated with fine-ground calcium carbonate and micro-nano-fibrillated cellulose, which was used as a binder and essential humectant to avoid formation of a stagnant air layer. Pre-oxidation countered the action of denitrification bacteria colonising the cellulose substrate. The by-product CO2 produced in situ during carbonate to nitrate conversion was adsorbed by perlite, which is an inert high surface-area additive. After use, the nitrate-rich CaCO3-cellulose-based filter was proposed to be mulched into a run-off resistant soil fertiliser and micronutrient suitable, e.g., for renewable forestry within the circular economy. Belgrade, Serbia, which is a highly polluted city, was used as a laboratory test bed, and NO2 was successfully removed from an inlet of city air. A construct of street-side self-draughting or municipal/commercial transport vehicle-exterior motion-draught filter boxes is discussed.
PB  - MDPI, Basel
T2  - Applied Sciences-Basel
T1  - Unveiling a Recycling-Sourced Mineral-Biocellulose Fibre Composite for Use in Combustion-Generated NOx Mitigation Forming Plant Nutrient: Meeting Sustainability Development Goals in the Circular Economy
IS  - 11
VL  - 10
DO  - 10.3390/app10113927
UR  - conv_6148
ER  - 
@article{
author = "Gane, Patrick and Dimić-Misić, Katarina and Barać, Nemanja and Imani, Monireh and Janaćković, Đorđe and Uskoković, Petar and Barcelo, Ernest",
year = "2020",
abstract = "Featured Application Surface flow filter for sorption of NOx in city/industrial pollution and conversion into a plant nutrient. Abstract NOx is unavoidably emitted during combustion in air at high temperature and/or pressure, which, if exceeding recommended levels, has a negative impact on the population. The authors found that when moist, limestone (CaCO3) readily sorbs NO2 to form calcium nitrate, which provides the basis for developing a surface flow filter. The substrate was made from "over-recycled" cellulose fibres such as newsprint, magazines, or packaging fibre, which are too weak to be used in further recycling. The substrate was specially-coated with fine-ground calcium carbonate and micro-nano-fibrillated cellulose, which was used as a binder and essential humectant to avoid formation of a stagnant air layer. Pre-oxidation countered the action of denitrification bacteria colonising the cellulose substrate. The by-product CO2 produced in situ during carbonate to nitrate conversion was adsorbed by perlite, which is an inert high surface-area additive. After use, the nitrate-rich CaCO3-cellulose-based filter was proposed to be mulched into a run-off resistant soil fertiliser and micronutrient suitable, e.g., for renewable forestry within the circular economy. Belgrade, Serbia, which is a highly polluted city, was used as a laboratory test bed, and NO2 was successfully removed from an inlet of city air. A construct of street-side self-draughting or municipal/commercial transport vehicle-exterior motion-draught filter boxes is discussed.",
publisher = "MDPI, Basel",
journal = "Applied Sciences-Basel",
title = "Unveiling a Recycling-Sourced Mineral-Biocellulose Fibre Composite for Use in Combustion-Generated NOx Mitigation Forming Plant Nutrient: Meeting Sustainability Development Goals in the Circular Economy",
number = "11",
volume = "10",
doi = "10.3390/app10113927",
url = "conv_6148"
}
Gane, P., Dimić-Misić, K., Barać, N., Imani, M., Janaćković, Đ., Uskoković, P.,& Barcelo, E.. (2020). Unveiling a Recycling-Sourced Mineral-Biocellulose Fibre Composite for Use in Combustion-Generated NOx Mitigation Forming Plant Nutrient: Meeting Sustainability Development Goals in the Circular Economy. in Applied Sciences-Basel
MDPI, Basel., 10(11).
https://doi.org/10.3390/app10113927
conv_6148
Gane P, Dimić-Misić K, Barać N, Imani M, Janaćković Đ, Uskoković P, Barcelo E. Unveiling a Recycling-Sourced Mineral-Biocellulose Fibre Composite for Use in Combustion-Generated NOx Mitigation Forming Plant Nutrient: Meeting Sustainability Development Goals in the Circular Economy. in Applied Sciences-Basel. 2020;10(11).
doi:10.3390/app10113927
conv_6148 .
Gane, Patrick, Dimić-Misić, Katarina, Barać, Nemanja, Imani, Monireh, Janaćković, Đorđe, Uskoković, Petar, Barcelo, Ernest, "Unveiling a Recycling-Sourced Mineral-Biocellulose Fibre Composite for Use in Combustion-Generated NOx Mitigation Forming Plant Nutrient: Meeting Sustainability Development Goals in the Circular Economy" in Applied Sciences-Basel, 10, no. 11 (2020),
https://doi.org/10.3390/app10113927 .,
conv_6148 .

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