Forced periodic operations of a chemical reactor for methanol synthesis - The search for the best scenario based on Nonlinear Frequency Response Method. Part II Simultaneous modulation of two inputs
Само за регистроване кориснике
2022
Аутори
Nikolic, DaliborkaSeidel, Carsten
Felischak, Matthias
Milicic, Tamara
Kienle, Achim
Seidel-Morgenstern, Andreas
Petkovska, Menka
Чланак у часопису (Објављена верзија)
Метаподаци
Приказ свих података о документуАпстракт
The analysis of the potential to improve performance of a methanol synthesis reactor through forced periodical operations by Nonlinear Frequency Response method is presented. The methanol synthesis in an isothermal and isobaric lab-scale CSTR is considered. First, the analysis was performed for single input modulations (in Part I), which showed that significant improvements can't be achieved. Here, the study is extended to analysis of simultaneous modulations of two inputs. All possible input combi-nations (6 cases) are analysed and the optimal forcing parameters, maximizing the time-average metha-nol production, were determined. For all combinations the improvement is possible, but for some cases it is not significant. The highest improvement is predicted for simultaneous modulation of the inlet partial pressure of CO and the inlet volumetric flow rate. This case, for which it is possible to achieve up to 33.51 % of methanol production, is analysed it detail and optimized using multi-...objective optimization.
Кључне речи:
Forced periodic operation / Methanol synthesis / Non-linear frequency response / Process improvement / Simultaneous modulation of two inputs / Multi-objective optimizationИзвор:
Chemical Engineering Science, 2022, 248Финансирање / пројекти:
- Министарство науке, технолошког развоја и иновација Републике Србије, институционално финансирање - 200135 (Универзитет у Београду, Технолошко-металуршки факултет) (RS-MESTD-inst-2020-200135)
DOI: 10.1016/j.ces.2021.117133
ISSN: 0009-2509
WoS: 000709895200002
Scopus: 2-s2.0-85116704542
Институција/група
Tehnološko-metalurški fakultetTY - JOUR AU - Nikolic, Daliborka AU - Seidel, Carsten AU - Felischak, Matthias AU - Milicic, Tamara AU - Kienle, Achim AU - Seidel-Morgenstern, Andreas AU - Petkovska, Menka PY - 2022 UR - http://TechnoRep.tmf.bg.ac.rs/handle/123456789/4973 AB - The analysis of the potential to improve performance of a methanol synthesis reactor through forced periodical operations by Nonlinear Frequency Response method is presented. The methanol synthesis in an isothermal and isobaric lab-scale CSTR is considered. First, the analysis was performed for single input modulations (in Part I), which showed that significant improvements can't be achieved. Here, the study is extended to analysis of simultaneous modulations of two inputs. All possible input combi-nations (6 cases) are analysed and the optimal forcing parameters, maximizing the time-average metha-nol production, were determined. For all combinations the improvement is possible, but for some cases it is not significant. The highest improvement is predicted for simultaneous modulation of the inlet partial pressure of CO and the inlet volumetric flow rate. This case, for which it is possible to achieve up to 33.51 % of methanol production, is analysed it detail and optimized using multi-objective optimization. T2 - Chemical Engineering Science T1 - Forced periodic operations of a chemical reactor for methanol synthesis - The search for the best scenario based on Nonlinear Frequency Response Method. Part II Simultaneous modulation of two inputs VL - 248 DO - 10.1016/j.ces.2021.117133 ER -
@article{ author = "Nikolic, Daliborka and Seidel, Carsten and Felischak, Matthias and Milicic, Tamara and Kienle, Achim and Seidel-Morgenstern, Andreas and Petkovska, Menka", year = "2022", abstract = "The analysis of the potential to improve performance of a methanol synthesis reactor through forced periodical operations by Nonlinear Frequency Response method is presented. The methanol synthesis in an isothermal and isobaric lab-scale CSTR is considered. First, the analysis was performed for single input modulations (in Part I), which showed that significant improvements can't be achieved. Here, the study is extended to analysis of simultaneous modulations of two inputs. All possible input combi-nations (6 cases) are analysed and the optimal forcing parameters, maximizing the time-average metha-nol production, were determined. For all combinations the improvement is possible, but for some cases it is not significant. The highest improvement is predicted for simultaneous modulation of the inlet partial pressure of CO and the inlet volumetric flow rate. This case, for which it is possible to achieve up to 33.51 % of methanol production, is analysed it detail and optimized using multi-objective optimization.", journal = "Chemical Engineering Science", title = "Forced periodic operations of a chemical reactor for methanol synthesis - The search for the best scenario based on Nonlinear Frequency Response Method. Part II Simultaneous modulation of two inputs", volume = "248", doi = "10.1016/j.ces.2021.117133" }
Nikolic, D., Seidel, C., Felischak, M., Milicic, T., Kienle, A., Seidel-Morgenstern, A.,& Petkovska, M.. (2022). Forced periodic operations of a chemical reactor for methanol synthesis - The search for the best scenario based on Nonlinear Frequency Response Method. Part II Simultaneous modulation of two inputs. in Chemical Engineering Science, 248. https://doi.org/10.1016/j.ces.2021.117133
Nikolic D, Seidel C, Felischak M, Milicic T, Kienle A, Seidel-Morgenstern A, Petkovska M. Forced periodic operations of a chemical reactor for methanol synthesis - The search for the best scenario based on Nonlinear Frequency Response Method. Part II Simultaneous modulation of two inputs. in Chemical Engineering Science. 2022;248. doi:10.1016/j.ces.2021.117133 .
Nikolic, Daliborka, Seidel, Carsten, Felischak, Matthias, Milicic, Tamara, Kienle, Achim, Seidel-Morgenstern, Andreas, Petkovska, Menka, "Forced periodic operations of a chemical reactor for methanol synthesis - The search for the best scenario based on Nonlinear Frequency Response Method. Part II Simultaneous modulation of two inputs" in Chemical Engineering Science, 248 (2022), https://doi.org/10.1016/j.ces.2021.117133 . .