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Novel membrane-supported hydrogel for removal of heavy metals

Authorized Users Only
2015
Authors
Stajčić, Aleksandar
Nastasović, Aleksandra
Stajić-Trošić, Jasna
Marković, Jelena P.
Onjia, Antonije
Radovanović, Filip
Article (Published version)
Metadata
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Abstract
Polyethersulfone membranes with integrated negatively-charged hydrogel of crosslinked poly (acrylamido-2-methylpropane sulfonic acid) were prepared by a combination of a liquid phase inversion process with photopolymerization and crosslinking of functional monomers included in the casting solution. A designed experiment was conducted to select the optimal composition for preparing membranes with a sufficient degree of swelling and ion exchange capacity. Scanning electron microscopy images revealed an ultrafine hybrid structure with an interconnected network of submicron particles embedded within the microporous polyethersulfone support. An intramembrane diffusion model was used to describe kinetics of heavy metal sorption by these hydrogels and the calculated apparent diffusion coefficients were 2-3 times larger than in commercial ion-exchange resins. Equilibrium sorption of heavy metals was described using a semi-empirical Langmuir model.
Keywords:
Membrane formation / Photoirradiation / Hydrogel / Heavy metal removal
Source:
Journal of Environmental Chemical Engineering, 2015, 3, 1, 453-461
Publisher:
  • Elsevier Sci Ltd, Oxford
Funding / projects:
  • Micro- Nanosystems and Sensors for Electric Power and Process Industry and Environmental Protection (RS-32008)
  • Advanced technologies for monitoring and environmental protection from chemical pollutants and radiation burden (RS-43009)

DOI: 10.1016/j.jece.2015.01.005

ISSN: 2213-3437

WoS: 000217976100054

Scopus: 2-s2.0-84961290325
[ Google Scholar ]
16
14
URI
http://TechnoRep.tmf.bg.ac.rs/handle/123456789/2917
Collections
  • Radovi istraživača / Researchers’ publications (TMF)
Institution/Community
Tehnološko-metalurški fakultet
TY  - JOUR
AU  - Stajčić, Aleksandar
AU  - Nastasović, Aleksandra
AU  - Stajić-Trošić, Jasna
AU  - Marković, Jelena P.
AU  - Onjia, Antonije
AU  - Radovanović, Filip
PY  - 2015
UR  - http://TechnoRep.tmf.bg.ac.rs/handle/123456789/2917
AB  - Polyethersulfone membranes with integrated negatively-charged hydrogel of crosslinked poly (acrylamido-2-methylpropane sulfonic acid) were prepared by a combination of a liquid phase inversion process with photopolymerization and crosslinking of functional monomers included in the casting solution. A designed experiment was conducted to select the optimal composition for preparing membranes with a sufficient degree of swelling and ion exchange capacity. Scanning electron microscopy images revealed an ultrafine hybrid structure with an interconnected network of submicron particles embedded within the microporous polyethersulfone support. An intramembrane diffusion model was used to describe kinetics of heavy metal sorption by these hydrogels and the calculated apparent diffusion coefficients were 2-3 times larger than in commercial ion-exchange resins. Equilibrium sorption of heavy metals was described using a semi-empirical Langmuir model.
PB  - Elsevier Sci Ltd, Oxford
T2  - Journal of Environmental Chemical Engineering
T1  - Novel membrane-supported hydrogel for removal of heavy metals
EP  - 461
IS  - 1
SP  - 453
VL  - 3
DO  - 10.1016/j.jece.2015.01.005
ER  - 
@article{
author = "Stajčić, Aleksandar and Nastasović, Aleksandra and Stajić-Trošić, Jasna and Marković, Jelena P. and Onjia, Antonije and Radovanović, Filip",
year = "2015",
abstract = "Polyethersulfone membranes with integrated negatively-charged hydrogel of crosslinked poly (acrylamido-2-methylpropane sulfonic acid) were prepared by a combination of a liquid phase inversion process with photopolymerization and crosslinking of functional monomers included in the casting solution. A designed experiment was conducted to select the optimal composition for preparing membranes with a sufficient degree of swelling and ion exchange capacity. Scanning electron microscopy images revealed an ultrafine hybrid structure with an interconnected network of submicron particles embedded within the microporous polyethersulfone support. An intramembrane diffusion model was used to describe kinetics of heavy metal sorption by these hydrogels and the calculated apparent diffusion coefficients were 2-3 times larger than in commercial ion-exchange resins. Equilibrium sorption of heavy metals was described using a semi-empirical Langmuir model.",
publisher = "Elsevier Sci Ltd, Oxford",
journal = "Journal of Environmental Chemical Engineering",
title = "Novel membrane-supported hydrogel for removal of heavy metals",
pages = "461-453",
number = "1",
volume = "3",
doi = "10.1016/j.jece.2015.01.005"
}
Stajčić, A., Nastasović, A., Stajić-Trošić, J., Marković, J. P., Onjia, A.,& Radovanović, F.. (2015). Novel membrane-supported hydrogel for removal of heavy metals. in Journal of Environmental Chemical Engineering
Elsevier Sci Ltd, Oxford., 3(1), 453-461.
https://doi.org/10.1016/j.jece.2015.01.005
Stajčić A, Nastasović A, Stajić-Trošić J, Marković JP, Onjia A, Radovanović F. Novel membrane-supported hydrogel for removal of heavy metals. in Journal of Environmental Chemical Engineering. 2015;3(1):453-461.
doi:10.1016/j.jece.2015.01.005 .
Stajčić, Aleksandar, Nastasović, Aleksandra, Stajić-Trošić, Jasna, Marković, Jelena P., Onjia, Antonije, Radovanović, Filip, "Novel membrane-supported hydrogel for removal of heavy metals" in Journal of Environmental Chemical Engineering, 3, no. 1 (2015):453-461,
https://doi.org/10.1016/j.jece.2015.01.005 . .

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