Origins of Polycyclic Aromatic Hydrocarbons in Sediments from the Danube and Sava Rivers and Their Tributaries in Serbia
Аутори
Crnković, DraganSekulić, Zoran
Antonović, Dušan
Marinković, Aleksandar
Popović, Slađana
Nikolić, Jasmina
Drmanić, Saša
Чланак у часопису (Објављена верзија)
Метаподаци
Приказ свих података о документуАпстракт
This study focussed on a comprehensive investigation on the state of pollution and identification of potential sources of contamination of some river sediments in Serbia by polycyclic aromatic hydrocarbons (PAHs), and is the basis for setting up further monitoring programs. The sediment quality of the Danube River (km 1433-845) and its tributaries in Serbia, including the Sava River (km 202-1), were analysed with respect to PAHs and total organic carbon (TOC). We found that total PAH concentration in the sediments from the Danube and its tributaries (10.0-4140 mu g kg(-1)) was lower than total PAH concentration in Sava River sediments (265.1-11272 mu g kg(-1)). Principal component analysis showed that concentrations of benzo[a]anthracene, chrysene, pyrene, fluoranthene, indeno[1,2,3- cd]pyrene, benzo[a] pyrene, benzo[b]fluoranthene and benzo[k]fluoranthene in the sediments were correlated with TOC. The diagnostic ratios anthracene/(anthracene+phenanthrene) and fluoranthene/(fluoranthen...e+ pyrene) were calculated to evaluate the emission sources of the PAHs. Therefore, these ratios indicated the predominantly pyrogenic source of the PAHs in the sediments. Results have also shown that river sediments in the Danube and Sava rivers and their tributaries were not recently polluted with PAHs, excluding only one location - S4, downstream of Sabac and characterized by heavily polluted sediment.
Кључне речи:
river sediment / PAHs / pollution sources / Danube River / Sava RiverИзвор:
Polish Journal of Environmental Studies, 2020, 29, 3, 2101-2110Издавач:
- Hard, Olsztyn 5
Финансирање / пројекти:
- Проучавање синтезе, структуре и активности органских једињења природног и синтетског порекла (RS-MESTD-Basic Research (BR or ON)-172013)
DOI: 10.15244/pjoes/111319
ISSN: 1230-1485
WoS: 000522535900010
Scopus: 2-s2.0-85083117790
Институција/група
Tehnološko-metalurški fakultetTY - JOUR AU - Crnković, Dragan AU - Sekulić, Zoran AU - Antonović, Dušan AU - Marinković, Aleksandar AU - Popović, Slađana AU - Nikolić, Jasmina AU - Drmanić, Saša PY - 2020 UR - http://TechnoRep.tmf.bg.ac.rs/handle/123456789/4460 AB - This study focussed on a comprehensive investigation on the state of pollution and identification of potential sources of contamination of some river sediments in Serbia by polycyclic aromatic hydrocarbons (PAHs), and is the basis for setting up further monitoring programs. The sediment quality of the Danube River (km 1433-845) and its tributaries in Serbia, including the Sava River (km 202-1), were analysed with respect to PAHs and total organic carbon (TOC). We found that total PAH concentration in the sediments from the Danube and its tributaries (10.0-4140 mu g kg(-1)) was lower than total PAH concentration in Sava River sediments (265.1-11272 mu g kg(-1)). Principal component analysis showed that concentrations of benzo[a]anthracene, chrysene, pyrene, fluoranthene, indeno[1,2,3- cd]pyrene, benzo[a] pyrene, benzo[b]fluoranthene and benzo[k]fluoranthene in the sediments were correlated with TOC. The diagnostic ratios anthracene/(anthracene+phenanthrene) and fluoranthene/(fluoranthene+ pyrene) were calculated to evaluate the emission sources of the PAHs. Therefore, these ratios indicated the predominantly pyrogenic source of the PAHs in the sediments. Results have also shown that river sediments in the Danube and Sava rivers and their tributaries were not recently polluted with PAHs, excluding only one location - S4, downstream of Sabac and characterized by heavily polluted sediment. PB - Hard, Olsztyn 5 T2 - Polish Journal of Environmental Studies T1 - Origins of Polycyclic Aromatic Hydrocarbons in Sediments from the Danube and Sava Rivers and Their Tributaries in Serbia EP - 2110 IS - 3 SP - 2101 VL - 29 DO - 10.15244/pjoes/111319 ER -
@article{ author = "Crnković, Dragan and Sekulić, Zoran and Antonović, Dušan and Marinković, Aleksandar and Popović, Slađana and Nikolić, Jasmina and Drmanić, Saša", year = "2020", abstract = "This study focussed on a comprehensive investigation on the state of pollution and identification of potential sources of contamination of some river sediments in Serbia by polycyclic aromatic hydrocarbons (PAHs), and is the basis for setting up further monitoring programs. The sediment quality of the Danube River (km 1433-845) and its tributaries in Serbia, including the Sava River (km 202-1), were analysed with respect to PAHs and total organic carbon (TOC). We found that total PAH concentration in the sediments from the Danube and its tributaries (10.0-4140 mu g kg(-1)) was lower than total PAH concentration in Sava River sediments (265.1-11272 mu g kg(-1)). Principal component analysis showed that concentrations of benzo[a]anthracene, chrysene, pyrene, fluoranthene, indeno[1,2,3- cd]pyrene, benzo[a] pyrene, benzo[b]fluoranthene and benzo[k]fluoranthene in the sediments were correlated with TOC. The diagnostic ratios anthracene/(anthracene+phenanthrene) and fluoranthene/(fluoranthene+ pyrene) were calculated to evaluate the emission sources of the PAHs. Therefore, these ratios indicated the predominantly pyrogenic source of the PAHs in the sediments. Results have also shown that river sediments in the Danube and Sava rivers and their tributaries were not recently polluted with PAHs, excluding only one location - S4, downstream of Sabac and characterized by heavily polluted sediment.", publisher = "Hard, Olsztyn 5", journal = "Polish Journal of Environmental Studies", title = "Origins of Polycyclic Aromatic Hydrocarbons in Sediments from the Danube and Sava Rivers and Their Tributaries in Serbia", pages = "2110-2101", number = "3", volume = "29", doi = "10.15244/pjoes/111319" }
Crnković, D., Sekulić, Z., Antonović, D., Marinković, A., Popović, S., Nikolić, J.,& Drmanić, S.. (2020). Origins of Polycyclic Aromatic Hydrocarbons in Sediments from the Danube and Sava Rivers and Their Tributaries in Serbia. in Polish Journal of Environmental Studies Hard, Olsztyn 5., 29(3), 2101-2110. https://doi.org/10.15244/pjoes/111319
Crnković D, Sekulić Z, Antonović D, Marinković A, Popović S, Nikolić J, Drmanić S. Origins of Polycyclic Aromatic Hydrocarbons in Sediments from the Danube and Sava Rivers and Their Tributaries in Serbia. in Polish Journal of Environmental Studies. 2020;29(3):2101-2110. doi:10.15244/pjoes/111319 .
Crnković, Dragan, Sekulić, Zoran, Antonović, Dušan, Marinković, Aleksandar, Popović, Slađana, Nikolić, Jasmina, Drmanić, Saša, "Origins of Polycyclic Aromatic Hydrocarbons in Sediments from the Danube and Sava Rivers and Their Tributaries in Serbia" in Polish Journal of Environmental Studies, 29, no. 3 (2020):2101-2110, https://doi.org/10.15244/pjoes/111319 . .