TechnoRep - Faculty of Technology and Metallurgy Repository
University of Belgrade - Faculty of Technology and Metallurgy
    • English
    • Српски
    • Српски (Serbia)
  • English 
    • English
    • Serbian (Cyrillic)
    • Serbian (Latin)
  • Login
View Item 
  •   TechnoRep
  • Tehnološko-metalurški fakultet
  • Radovi istraživača / Researchers’ publications (TMF)
  • View Item
  •   TechnoRep
  • Tehnološko-metalurški fakultet
  • Radovi istraživača / Researchers’ publications (TMF)
  • View Item
JavaScript is disabled for your browser. Some features of this site may not work without it.

Forced Periodic Operation of Methanol Synthesis in an Isothermal Gradientless Reactor

Authorized Users Only
2022
Authors
Seidel, Carsten
Nikolić, Daliborka
Felischak, Matthias
Petkovska, Menka
Seidel-Morgenstern, Andreas
Kienle, Achim
Article (Published version)
Metadata
Show full item record
Abstract
Methanol synthesis from synthesis gas with heterogeneous Cu/ZnO/Al2O3 catalysts in an isothermal gradientless reactor is described. In a theoretical study, the potential of forced periodic operation (FPO) for improving reactor performance in terms of methanol production rate and methanol yield is explored. The approach is based on a detailed kinetic model and combines nonlinear frequency response (NFR) analysis with rigorous numerical multi-objective optimization. Optimal steady-state operation is compared with optimal forced periodic operation for a given benchmark problem with and without inert nitrogen in the feed. Further, the significant influence of the saturation capacity of the solid phase on the dynamic behavior in response to step changes and periodic input modulations is studied.
Keywords:
Forced periodic operation / Methanol synthesis / Multi-objective optimization / Nonlinear frequency response / Pareto fronts
Source:
Chemical Engineering and Technology, 2022
Publisher:
  • John Wiley and Sons Inc
Funding / projects:
  • Financial support by the German Research Foundation (DFG) is gratefully acknowledged through the priority program SPP 2080 under grant KI 417/6‐2, NI 2222/1‐2, SE 586/24‐2.

DOI: 10.1002/ceat.202200286

ISSN: 0930-7516

Scopus: 2-s2.0-85141538190
[ Google Scholar ]
1
URI
http://TechnoRep.tmf.bg.ac.rs/handle/123456789/5267
Collections
  • Radovi istraživača / Researchers’ publications (TMF)
Institution/Community
Tehnološko-metalurški fakultet
TY  - JOUR
AU  - Seidel, Carsten
AU  - Nikolić, Daliborka
AU  - Felischak, Matthias
AU  - Petkovska, Menka
AU  - Seidel-Morgenstern, Andreas
AU  - Kienle, Achim
PY  - 2022
UR  - http://TechnoRep.tmf.bg.ac.rs/handle/123456789/5267
AB  - Methanol synthesis from synthesis gas with heterogeneous Cu/ZnO/Al2O3 catalysts in an isothermal gradientless reactor is described. In a theoretical study, the potential of forced periodic operation (FPO) for improving reactor performance in terms of methanol production rate and methanol yield is explored. The approach is based on a detailed kinetic model and combines nonlinear frequency response (NFR) analysis with rigorous numerical multi-objective optimization. Optimal steady-state operation is compared with optimal forced periodic operation for a given benchmark problem with and without inert nitrogen in the feed. Further, the significant influence of the saturation capacity of the solid phase on the dynamic behavior in response to step changes and periodic input modulations is studied.
PB  - John Wiley and Sons Inc
T2  - Chemical Engineering and Technology
T1  - Forced Periodic Operation of Methanol Synthesis in an Isothermal Gradientless Reactor
DO  - 10.1002/ceat.202200286
ER  - 
@article{
author = "Seidel, Carsten and Nikolić, Daliborka and Felischak, Matthias and Petkovska, Menka and Seidel-Morgenstern, Andreas and Kienle, Achim",
year = "2022",
abstract = "Methanol synthesis from synthesis gas with heterogeneous Cu/ZnO/Al2O3 catalysts in an isothermal gradientless reactor is described. In a theoretical study, the potential of forced periodic operation (FPO) for improving reactor performance in terms of methanol production rate and methanol yield is explored. The approach is based on a detailed kinetic model and combines nonlinear frequency response (NFR) analysis with rigorous numerical multi-objective optimization. Optimal steady-state operation is compared with optimal forced periodic operation for a given benchmark problem with and without inert nitrogen in the feed. Further, the significant influence of the saturation capacity of the solid phase on the dynamic behavior in response to step changes and periodic input modulations is studied.",
publisher = "John Wiley and Sons Inc",
journal = "Chemical Engineering and Technology",
title = "Forced Periodic Operation of Methanol Synthesis in an Isothermal Gradientless Reactor",
doi = "10.1002/ceat.202200286"
}
Seidel, C., Nikolić, D., Felischak, M., Petkovska, M., Seidel-Morgenstern, A.,& Kienle, A.. (2022). Forced Periodic Operation of Methanol Synthesis in an Isothermal Gradientless Reactor. in Chemical Engineering and Technology
John Wiley and Sons Inc..
https://doi.org/10.1002/ceat.202200286
Seidel C, Nikolić D, Felischak M, Petkovska M, Seidel-Morgenstern A, Kienle A. Forced Periodic Operation of Methanol Synthesis in an Isothermal Gradientless Reactor. in Chemical Engineering and Technology. 2022;.
doi:10.1002/ceat.202200286 .
Seidel, Carsten, Nikolić, Daliborka, Felischak, Matthias, Petkovska, Menka, Seidel-Morgenstern, Andreas, Kienle, Achim, "Forced Periodic Operation of Methanol Synthesis in an Isothermal Gradientless Reactor" in Chemical Engineering and Technology (2022),
https://doi.org/10.1002/ceat.202200286 . .

DSpace software copyright © 2002-2015  DuraSpace
About TechnoRep | Send Feedback

OpenAIRERCUB
 

 

All of DSpaceInstitutions/communitiesAuthorsTitlesSubjectsThis institutionAuthorsTitlesSubjects

Statistics

View Usage Statistics

DSpace software copyright © 2002-2015  DuraSpace
About TechnoRep | Send Feedback

OpenAIRERCUB