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dc.creatorSeidel, Carsten
dc.creatorNikolić, Daliborka
dc.creatorFelischak, Matthias
dc.creatorPetkovska, Menka
dc.creatorSeidel-Morgenstern, Andreas
dc.creatorKienle, Achim
dc.date.accessioned2022-12-07T14:00:58Z
dc.date.available2022-12-07T14:00:58Z
dc.date.issued2022
dc.identifier.issn0930-7516
dc.identifier.urihttp://TechnoRep.tmf.bg.ac.rs/handle/123456789/5267
dc.description.abstractMethanol synthesis from synthesis gas with heterogeneous Cu/ZnO/Al2O3 catalysts in an isothermal gradientless reactor is described. In a theoretical study, the potential of forced periodic operation (FPO) for improving reactor performance in terms of methanol production rate and methanol yield is explored. The approach is based on a detailed kinetic model and combines nonlinear frequency response (NFR) analysis with rigorous numerical multi-objective optimization. Optimal steady-state operation is compared with optimal forced periodic operation for a given benchmark problem with and without inert nitrogen in the feed. Further, the significant influence of the saturation capacity of the solid phase on the dynamic behavior in response to step changes and periodic input modulations is studied.sr
dc.language.isoensr
dc.publisherJohn Wiley and Sons Incsr
dc.relationFinancial support by the German Research Foundation (DFG) is gratefully acknowledged through the priority program SPP 2080 under grant KI 417/6‐2, NI 2222/1‐2, SE 586/24‐2.sr
dc.rightsrestrictedAccesssr
dc.sourceChemical Engineering and Technologysr
dc.subjectForced periodic operationsr
dc.subjectMethanol synthesissr
dc.subjectMulti-objective optimizationsr
dc.subjectNonlinear frequency responsesr
dc.subjectPareto frontssr
dc.titleForced Periodic Operation of Methanol Synthesis in an Isothermal Gradientless Reactorsr
dc.typearticlesr
dc.rights.licenseARRsr
dc.citation.rankM23~
dc.identifier.doi10.1002/ceat.202200286
dc.identifier.scopus2-s2.0-85141538190
dc.type.versionpublishedVersionsr


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