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Occurrence and behavior of selected pharmaceuticals during riverbank filtration in The Republic of Serbia

Authorized Users Only
2017
Authors
Kovačević, Srđan
Radišić, Marina
Laušević, Mila
Dimkić, Milan
Article (Published version)
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Abstract
The objectives of the research are to determine the occurrence of pharmaceuticals in surface water and groundwater in the Republic of Serbia and to identify significant effects of river-water purification through riverbank filtration, concerning oxic conditions and hydrogeological conditions of alluvial aquifers in Serbia. Between 2009 and 2015, a total of 19 studied pharmaceuticals and metabolites were analyzed in 184 samples, 10 were detected in surface water, and 8 in groundwater. Carbamazepine and metamizole metabolites N-acetyl-4-amino-antipyrine (4-AAA) and N-formyl-4-amino-antipyrine (4-FAA) have the highest frequency of occurrence in surface water (57.3–68.8 %) and in groundwater (19.5–43.9 %), respectively. Highest detected concentrations were for 4-AAA (520 ng/L) and 4-FAA (248 ng/L) in surface water as well as in groundwater (4-AAA 128 ng/L and 4-FAA 150 ng/L). Results showed that riverbank filtration sites with different hydrogeological and oxic conditions could significant...ly remove investigated pharmaceuticals. Percentage of removal during riverbank filtration was determined for carbamazepine (65.4 %), trimethoprim (100 %), 4-AAA (91.2 %), and 4-FAA (70 %) for all investigated locations. Based on the available data for three specific locations (Danube River alluvion, Sava River alluvion, and Velika Morava River alluvion), results showed that besides oxic conditions, residence time of groundwater in alluvial aquifer and ratio of infiltrated water from river to the well play very important role in the quality of groundwater. These results are extremely important for better understanding of self-purification potential of alluvial aquifers and protection from potential impacts of anthropogenic pollution to the groundwater sources in the Republic of Serbia.

Keywords:
Groundwater / Occurrence / Pharmaceuticals / Riverbank filtration / Surface water
Source:
Environmental Science and Pollution Research, 2017, 24, 2, 2075-2088
Publisher:
  • Springer Verlag
Funding / projects:
  • Ministry of Science and Technological Development (TR37104).
  • Development and Application of Methods and Materials for Monitoring New Organic Contaminants, Toxic Compounds and Heavy Metals (RS-172007)
  • The project "Study of Well Ageing and Maintenance" of the Ministry of Agriculture, Forestry and Water Management/National Water Directorate.

DOI: 10.1007/s11356-016-7959-4

ISSN: 0944-1344

WoS: 000394254000090

Scopus: 2-s2.0-84994336699
[ Google Scholar ]
28
7
URI
http://TechnoRep.tmf.bg.ac.rs/handle/123456789/5835
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  • Radovi istraživača (Inovacioni centar) / Researchers’ publications (Innovation Centre)
  • Radovi istraživača / Researchers’ publications (TMF)
Institution/Community
Inovacioni centar
TY  - JOUR
AU  - Kovačević, Srđan
AU  - Radišić, Marina
AU  - Laušević, Mila
AU  - Dimkić, Milan
PY  - 2017
UR  - http://TechnoRep.tmf.bg.ac.rs/handle/123456789/5835
AB  - The objectives of the research are to determine the occurrence of pharmaceuticals in surface water and groundwater in the Republic of Serbia and to identify significant effects of river-water purification through riverbank filtration, concerning oxic conditions and hydrogeological conditions of alluvial aquifers in Serbia. Between 2009 and 2015, a total of 19 studied pharmaceuticals and metabolites were analyzed in 184 samples, 10 were detected in surface water, and 8 in groundwater. Carbamazepine and metamizole metabolites N-acetyl-4-amino-antipyrine (4-AAA) and N-formyl-4-amino-antipyrine (4-FAA) have the highest frequency of occurrence in surface water (57.3–68.8 %) and in groundwater (19.5–43.9 %), respectively. Highest detected concentrations were for 4-AAA (520 ng/L) and 4-FAA (248 ng/L) in surface water as well as in groundwater (4-AAA 128 ng/L and 4-FAA 150 ng/L). Results showed that riverbank filtration sites with different hydrogeological and oxic conditions could significantly remove investigated pharmaceuticals. Percentage of removal during riverbank filtration was determined for carbamazepine (65.4 %), trimethoprim (100 %), 4-AAA (91.2 %), and 4-FAA (70 %) for all investigated locations. Based on the available data for three specific locations (Danube River alluvion, Sava River alluvion, and Velika Morava River alluvion), results showed that besides oxic conditions, residence time of groundwater in alluvial aquifer and ratio of infiltrated water from river to the well play very important role in the quality of groundwater. These results are extremely important for better understanding of self-purification potential of alluvial aquifers and protection from potential impacts of anthropogenic pollution to the groundwater sources in the Republic of Serbia.
PB  - Springer Verlag
T2  - Environmental Science and Pollution Research
T1  - Occurrence and behavior of selected pharmaceuticals during riverbank filtration in The Republic of Serbia
EP  - 2088
IS  - 2
SP  - 2075
VL  - 24
DO  - 10.1007/s11356-016-7959-4
ER  - 
@article{
author = "Kovačević, Srđan and Radišić, Marina and Laušević, Mila and Dimkić, Milan",
year = "2017",
abstract = "The objectives of the research are to determine the occurrence of pharmaceuticals in surface water and groundwater in the Republic of Serbia and to identify significant effects of river-water purification through riverbank filtration, concerning oxic conditions and hydrogeological conditions of alluvial aquifers in Serbia. Between 2009 and 2015, a total of 19 studied pharmaceuticals and metabolites were analyzed in 184 samples, 10 were detected in surface water, and 8 in groundwater. Carbamazepine and metamizole metabolites N-acetyl-4-amino-antipyrine (4-AAA) and N-formyl-4-amino-antipyrine (4-FAA) have the highest frequency of occurrence in surface water (57.3–68.8 %) and in groundwater (19.5–43.9 %), respectively. Highest detected concentrations were for 4-AAA (520 ng/L) and 4-FAA (248 ng/L) in surface water as well as in groundwater (4-AAA 128 ng/L and 4-FAA 150 ng/L). Results showed that riverbank filtration sites with different hydrogeological and oxic conditions could significantly remove investigated pharmaceuticals. Percentage of removal during riverbank filtration was determined for carbamazepine (65.4 %), trimethoprim (100 %), 4-AAA (91.2 %), and 4-FAA (70 %) for all investigated locations. Based on the available data for three specific locations (Danube River alluvion, Sava River alluvion, and Velika Morava River alluvion), results showed that besides oxic conditions, residence time of groundwater in alluvial aquifer and ratio of infiltrated water from river to the well play very important role in the quality of groundwater. These results are extremely important for better understanding of self-purification potential of alluvial aquifers and protection from potential impacts of anthropogenic pollution to the groundwater sources in the Republic of Serbia.",
publisher = "Springer Verlag",
journal = "Environmental Science and Pollution Research",
title = "Occurrence and behavior of selected pharmaceuticals during riverbank filtration in The Republic of Serbia",
pages = "2088-2075",
number = "2",
volume = "24",
doi = "10.1007/s11356-016-7959-4"
}
Kovačević, S., Radišić, M., Laušević, M.,& Dimkić, M.. (2017). Occurrence and behavior of selected pharmaceuticals during riverbank filtration in The Republic of Serbia. in Environmental Science and Pollution Research
Springer Verlag., 24(2), 2075-2088.
https://doi.org/10.1007/s11356-016-7959-4
Kovačević S, Radišić M, Laušević M, Dimkić M. Occurrence and behavior of selected pharmaceuticals during riverbank filtration in The Republic of Serbia. in Environmental Science and Pollution Research. 2017;24(2):2075-2088.
doi:10.1007/s11356-016-7959-4 .
Kovačević, Srđan, Radišić, Marina, Laušević, Mila, Dimkić, Milan, "Occurrence and behavior of selected pharmaceuticals during riverbank filtration in The Republic of Serbia" in Environmental Science and Pollution Research, 24, no. 2 (2017):2075-2088,
https://doi.org/10.1007/s11356-016-7959-4 . .

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